globalchange  > 气候变化事实与影响
DOI: 10.5194/acp-19-4877-2019
WOS记录号: WOS:000464163000003
论文题名:
Exploring accumulation-mode H2SO4 versus SO2 stratospheric sulfate geoengineering in a sectional aerosol-chemistry-climate model
作者: Vattioni, Sandro1,2; Weisenstein, Debra2; Keith, David2; Feinberg, Aryeh1; Peter, Thomas1; Stenke, Andrea1
通讯作者: Vattioni, Sandro
刊名: ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN: 1680-7316
EISSN: 1680-7324
出版年: 2019
卷: 19, 期:7, 页码:4877-4897
语种: 英语
WOS关键词: GENERAL-CIRCULATION MODEL ; TRANSPORT ; SENSITIVITY ; INJECTION ; MODULE ; SOCOL ; LIFETIME ; IMPACT ; SALSA
WOS学科分类: Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向: Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
英文摘要:

Stratospheric sulfate geoengineering (SSG) could contribute to avoiding some of the adverse impacts of climate change. We used the SOCOL-AER global aerosol-chemistry-climate model to investigate 21 different SSG scenarios, each with 1.83 Mt S yr(-1) injected either in the form of accumulation-mode H2SO4 droplets (AM H2SO4), gas-phase SO2 or as combinations of both. For most scenarios, the sulfur was continuously emitted at an altitude of 50 hPa (approximate to 20 km) in the tropics and subtropics. We assumed emissions to be zonally and latitudinally symmetric around the Equator. The spread of emissions ranged from 3.75 degrees S-3.75 degrees N to 30 degrees S-30 degrees N. In the SO2 emission scenarios, continuous production of tiny nucleation-mode particles results in increased coagulation, which together with gaseous H2SO4 condensation, produces coarse-mode particles. These large particles are less effective for backscattering solar radiation and have a shorter stratospheric residence time than AM H2SO4 particles. On average, the stratospheric aerosol burden and corresponding all-sky shortwave radiative forcing for the AM H2SO4 scenarios are about 37% larger than for the SO2 scenarios. The simulated stratospheric aerosol burdens show a weak dependence on the latitudinal spread of emissions. Emitting at 30 degrees N-30 degrees S instead of 10 degrees N-10 degrees S only decreases stratospheric burdens by about 10 %. This is because a decrease in coagulation and the resulting smaller particle size is roughly balanced by faster removal through stratosphere-to-troposphere transport via tropopause folds. Increasing the injection altitude is also ineffective, although it generates a larger stratospheric burden, because enhanced condensation and/or coagulation leads to larger particles, which are less effective scatterers. In the case of gaseous SO2 emissions, limiting the sulfur injections spatially and temporally in the form of point and pulsed emissions reduces the total global annual nucleation, leading to less coagulation and thus smaller particles with increased stratospheric residence times. Pulse or point emissions of AM H2SO4 have the opposite effect: they decrease the stratospheric aerosol burden by increasing coagulation and only slightly decrease clear-sky radiative forcing. This study shows that direct emission of AM H2SO4 results in higher radiative forcing for the same sulfur equivalent mass injection strength than SO2 emissions, and that the sensitivity to different injection strategies varies for different forms of injected sulfur.


Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/134232
Appears in Collections:气候变化事实与影响

Files in This Item:

There are no files associated with this item.


作者单位: 1.Swiss Fed Inst Technol, Inst Atmospher & Climate Sci, CH-8092 Zurich, Switzerland
2.Harvard John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA

Recommended Citation:
Vattioni, Sandro,Weisenstein, Debra,Keith, David,et al. Exploring accumulation-mode H2SO4 versus SO2 stratospheric sulfate geoengineering in a sectional aerosol-chemistry-climate model[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019-01-01,19(7):4877-4897
Service
Recommend this item
Sava as my favorate item
Show this item's statistics
Export Endnote File
Google Scholar
Similar articles in Google Scholar
[Vattioni, Sandro]'s Articles
[Weisenstein, Debra]'s Articles
[Keith, David]'s Articles
百度学术
Similar articles in Baidu Scholar
[Vattioni, Sandro]'s Articles
[Weisenstein, Debra]'s Articles
[Keith, David]'s Articles
CSDL cross search
Similar articles in CSDL Cross Search
[Vattioni, Sandro]‘s Articles
[Weisenstein, Debra]‘s Articles
[Keith, David]‘s Articles
Related Copyright Policies
Null
收藏/分享
所有评论 (0)
暂无评论
 

Items in IR are protected by copyright, with all rights reserved, unless otherwise indicated.