globalchange  > 影响、适应和脆弱性
DOI: 10.1088/1748-9326/11/4/044010
论文题名:
Evaluating ethane and methane emissions associated with the development of oil and natural gas extraction in North America
作者: B Franco; E Mahieu; L K Emmons; Z A Tzompa-Sosa; E V Fischer; K Sudo; B Bovy; S Conway; D Griffin; J W Hannigan; K Strong; K A Walker
刊名: Environmental Research Letters
ISSN: 1748-9326
出版年: 2016
发表日期: 2016-04-07
卷: 11, 期:4
语种: 英语
英文摘要:

Sharp rises in the atmospheric abundance of ethane (C2H6) have been detected from 2009 onwards in the Northern Hemisphere as a result of the unprecedented growth in the exploitation of shale gas and tight oil reservoirs in North America. Using time series of C2H6 total columns derived from ground-based Fourier transform infrared (FTIR) observations made at five selected Network for the Detection of Atmospheric Composition Change sites, we characterize the recent C2H6 evolution and determine growth rates of ~5% yr−1 at mid-latitudes and of ~3% yr−1 at remote sites. Results from CAM-chem simulations with the Hemispheric Transport of Air Pollutants, Phase II bottom-up inventory for anthropogenic emissions are found to greatly underestimate the current C2H6 abundances. Doubling global emissions is required to reconcile the simulations and the observations prior to 2009. We further estimate that North American anthropogenic C2H6 emissions have increased from 1.6 Tg yr−1 in 2008 to 2.8 Tg yr−1 in 2014, i.e. by 75% over these six years. We also completed a second simulation with new top-down emissions of C2H6 from North American oil and gas activities, biofuel consumption and biomass burning, inferred from space-borne observations of methane (CH4) from Greenhouse Gases Observing SATellite. In this simulation, GEOS-Chem is able to reproduce FTIR measurements at the mid-latitudinal sites, underscoring the impact of the North American oil and gas development on the current C2H6 abundance. Finally we estimate that the North American oil and gas emissions of CH4, a major greenhouse gas, grew from 20 to 35 Tg yr−1 over the period 2008–2014, in association with the recent C2H6 rise.

URL: http://iopscience.iop.org/article/10.1088/1748-9326/11/4/044010
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/13744
Appears in Collections:影响、适应和脆弱性
气候减缓与适应

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作者单位: Institute of Astrophysics and Geophysics, University of Liège, Liège, Belgium;Institute of Astrophysics and Geophysics, University of Liège, Liège, Belgium;National Center for Atmospheric Research, Boulder, CO, USA;Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA;Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA;Graduate School of Environmental Studies, Nagoya University, Nagoya, Japan;Department of Environmental Geochemical Cycle Research, Japan Agency for Marine-Earth Science and Technology, Yokohama, Japan;Institute of Astrophysics and Geophysics, University of Liège, Liège, Belgium;Department of Physics, University of Toronto, Toronto, ON, Canada;Department of Physics, University of Toronto, Toronto, ON, Canada;National Center for Atmospheric Research, Boulder, CO, USA;Department of Physics, University of Toronto, Toronto, ON, Canada;Department of Physics, University of Toronto, Toronto, ON, Canada;Department of Chemistry, University of Waterloo, Waterloo, ON, Canada

Recommended Citation:
B Franco,E Mahieu,L K Emmons,et al. Evaluating ethane and methane emissions associated with the development of oil and natural gas extraction in North America[J]. Environmental Research Letters,2016-01-01,11(4)
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