DOI: 10.1016/j.atmosenv.2020.117384
论文题名: Vertical distributions of tropospheric formaldehyde, nitrogen dioxide, ozone and aerosol in southern China by ground-based MAX-DOAS and LIDAR measurements during PRIDE-GBA 2018 campaign
作者: Luo Y. ; Dou K. ; Fan G. ; Huang S. ; Si F. ; Zhou H. ; Wang Y. ; Pei C. ; Tang F. ; Yang D. ; Xi L. ; Yang T. ; Zhang T. ; Liu W.
刊名: Atmospheric Environment
ISSN: 1352-2310
出版年: 2020
卷: 226 语种: 英语
英文关键词: Absorption spectroscopy
; Aerosols
; Formaldehyde
; Light absorption
; Nitrogen oxides
; Optical radar
; Ozone
; Photochemical forming
; Reaction intermediates
; Remote sensing
; Troposphere
; MAX-DOAS
; Precursor
; Tropospheric ozone
; Validation
; Vertical profile
; Air pollution
; formaldehyde
; nitrogen dioxide
; ozone
; radical
; volatile organic compound
; aerosol
; atmospheric pollution
; formaldehyde
; lidar
; megacity
; nitrogen dioxide
; oxidation
; ozone
; remote sensing
; troposphere
; vertical distribution
; absorption spectroscopy
; aerosol
; air pollution
; air quality
; Article
; China
; concentration (parameter)
; electric power plant
; industrial area
; light absorption
; measurement accuracy
; meteorology
; oxidation
; photochemistry
; pollution monitoring
; priority journal
; reliability
; remote sensing
; residential area
; traffic and transport
学科: Aerosol
; MAX-DOAS
; Precursor
; Tropospheric ozone
; Validation
; Vertical profile
中文摘要: As the development of megacities, combined air pollution has been of increasing concern in China, which is composed by primary pollution, such as Nitrogen dioxide (NO2), and the followed secondary pollution under certain meteorology circumstances and high concentration of precursors, such as tropospheric ozone, formaldehyde (HCHO) and fine particles. During PRIDE-GBA 2018 Campaign (Particles, Radicals, Intermediates from oxiDation of primary Emissions in Great Bay Area), we performed the high resolution vertical observations of pollution gases and aerosol, which are significant but scarce indexes in studying the mechanisms of tropospheric pollution, using remote sensing techniques. NO2 and HCHO column densities and vertical profiles are reconstructed from data of multi-axis differential optical absorption spectroscopy (MAX-DOAS). Tropospheric ozone profile and aerosol extinction are retrieved by the differential absorption light detection and ranging (LIDAR) system. In order to verifying the accuracy, we evaluated the consistency and reliability of MAX-DOAS and LIDAR measurements. The results showed reasonable agreement with in-situ and off-line observations at Canton Tower. A typical combined pollution process from Sep 29 to Oct 10 was analyzed in detail. More than 200 μg/m3 tropospheric ozone in this case was considered from the anthropogenic sources, including industry, power plant, residential and transportation. The high emission from local industry and polluted air transport from northeast brought the main precursors of this pollution process. The photochemical formation of tropospheric ozone was turned into a VOC-limited regime on polluted days. © 2020 Elsevier Ltd
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/160870
Appears in Collections: 气候变化与战略
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作者单位: Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, China; Institute for Environmental and Climate Research, Jinan University, Guangzhou, 510632, China; Guangzhou Environmental Monitoring Center, Guangzhou, 510060, China
Recommended Citation:
Luo Y.,Dou K.,Fan G.,et al. Vertical distributions of tropospheric formaldehyde, nitrogen dioxide, ozone and aerosol in southern China by ground-based MAX-DOAS and LIDAR measurements during PRIDE-GBA 2018 campaign[J]. Atmospheric Environment,2020-01-01,226