DOI: 10.1016/j.atmosenv.2015.01.021
Scopus记录号: 2-s2.0-84921854113
论文题名: Diurnal, seasonal, and annual trends in atmospheric CO2 at southwest London during 2000-2012: Wind sector analysis and comparison with Mace Head, Ireland
作者: Hernández-Paniagua I ; Y ; , Lowry D ; , Clemitshaw K ; C ; , Fisher R ; E ; , France J ; L ; , Lanoisellé M ; , Ramonet M ; , Nisbet E ; G
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2015
卷: 105 起始页码: 138
结束页码: 147
语种: 英语
英文关键词: Carbon dioxide
; Long-term trend
; Seasonal variation
Scopus关键词: Bioactivity
; Combustion
; Gas emissions
; Greenhouse gases
; Growth rate
; Anthropogenic emissions
; Combustion emissions
; Different time scale
; Greenhouse gas inventory
; Long-term trend
; Meteorological analysis
; Seasonal variation
; University of London
; Carbon dioxide
; atmospheric carbon dioxide
; carbon dioxide
; unclassified drug
; air mass
; annual variation
; anthropogenic effect
; atmospheric pollution
; carbon dioxide
; comparative study
; diurnal variation
; emission inventory
; global change
; long-term change
; NOAA satellite
; pollutant transport
; seasonal variation
; spatiotemporal analysis
; Article
; calibration
; carbon footprint
; circadian rhythm
; circannual rhythm
; combustion
; comparative study
; greenhouse gas
; growing season
; growth rate
; Ireland
; meteorology
; priority journal
; seasonal variation
; temperature
; United Kingdom
; wind
; Connacht
; County Galway
; England
; Ireland
; London [England]
; Mace Head
; United Kingdom
Scopus学科分类: Environmental Science: Water Science and Technology
; Earth and Planetary Sciences: Earth-Surface Processes
; Environmental Science: Environmental Chemistry
英文摘要: In-situ measurements of atmospheric CO2 have been made at Royal Holloway University of London (RHUL) in Egham (EGH), Surrey, UK from 2000 to 2012. The data were linked to the global scale using NOAA-calibrated gases. Measured CO2 varies on time scales that range from minutes to inter-annual and annual cycles. Seasonality and pollution episodes occur each year. Diurnal cycles vary with daylight and temperature, which influence the biological cycle of CO2 and the degree of vertical mixing. Anthropogenic emissions of CO2 dominate the variability during weekdays when transport cycles are greater than at weekends. Seasonal cycles are driven by temporal variations in biological activity and changes in combustion emissions. Maximum mole fractions (μmol/mol) (henceforth referred to by parts per million, ppm) occur in winter, with minima in late summer. The smallest seasonal amplitude observed, peak to trough, was 17.0ppm CO2 in 2003, whereas the largest amplitude observed was 27.1ppm CO2 in 2008.Meteorology can strongly modify the CO2 mole fractions at different time scales. Analysis of eight 45° wind sectors shows that the highest CO2 mole fractions were recorded from the E and SE sectors. Lowest mole fractions were observed for air masses from the S and SW. Back-trajectory and meteorological analyses of the data confirm that the dominant sources of CO2 are anthropogenic emissions from London and SE England. The largest annual rate of increase in the annual average of CO2, 3.26ppmyr-1 (p<0.05), was for the W sector with a smaller increase, 2.56ppmyr-1 (p<0.05), for the E sector. Calm winds showed an annual growth rate of 1.16ppmyr-1 CO2 (p<0.05) implying declining local sources. The EGH site shows an average growth rate of 2.5ppmyr-1 CO2 (p<0.05) over the measured period, which exceeds the observed global trend and contrasts with the decrease in CO2 emissions reported in UK greenhouse gas inventories. This is presumably because the region has had higher growth in combustion emissions than the global average, though the low growth rate in calm weather implies the local emissions have grown more slowly. The seasonal cycle at EGH had larger amplitudes than those recorded at the Mace Head Atmospheric Research Station (MHD) on the W coast of Ireland. Overall, the growth rate observed in annual average CO2 at EGH was larger than that at MHD by about 0.5ppmyr-1. © 2015 Elsevier Ltd. Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/81959
Appears in Collections: 气候变化事实与影响
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作者单位: Department of Earth Sciences, Royal Holloway, University of London, Egham, Surrey, United Kingdom; School of Environmental Sciences, University of East Anglia, Norwich, United Kingdom; Laboratoire des Sciences du Climat et de l'Environnement (LSCE/IPSL) CEA-CNRS-UVSQ, Gif-sur-Yvette, France
Recommended Citation:
Hernández-Paniagua I,Y,, Lowry D,et al. Diurnal, seasonal, and annual trends in atmospheric CO2 at southwest London during 2000-2012: Wind sector analysis and comparison with Mace Head, Ireland[J]. Atmospheric Environment,2015-01-01,105