DOI: | 10.1016/j.watres.2018.03.041
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Scopus记录号: | 2-s2.0-85044146069
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论文题名: | Removal of organic compounds from shale gas flowback water |
作者: | Butkovskyi A.; Faber A.-H.; Wang Y.; Grolle K.; Hofman-Caris R.; Bruning H.; Van Wezel A.P.; Rijnaarts H.H.M.
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刊名: | Water Research
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ISSN: | 431354
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出版年: | 2018
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卷: | 138 | 起始页码: | 47
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结束页码: | 55
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语种: | 英语
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英文关键词: | Aerobic degradation
; Dissolved organic carbon
; Flowback water
; Hydraulic fracturing
; Shale gas
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Scopus关键词: | Activated carbon
; Activated carbon treatment
; Chemical oxygen demand
; Desalination
; Dissolution
; Flotation
; Hydraulic fracturing
; Molecular weight
; Ozone
; Ozone water treatment
; Ozonization
; Shale
; Shale gas
; Stream flow
; Aerobic degradation
; Dissolved air floatations
; Dissolved air flotations
; Dissolved organic carbon
; Flowback
; Granular activated carbons
; Individual organic compounds
; Organic carbon fraction
; Organic carbon
; acid
; activated carbon
; ammonia
; carbon
; flowback water
; hydrogen
; nitrogen
; organic carbon
; organic compound
; oxygen
; phosphorus
; unclassified drug
; volatile fatty acid
; water
; charcoal
; natural gas
; organic compound
; ozone
; activated carbon
; anaerobic digestion
; chemical oxygen demand
; concentration (composition)
; dissolution
; dissolved organic carbon
; hydraulic fracturing
; inorganic compound
; ozonation
; pollutant removal
; shale gas
; sorption
; activated sludge
; adsorption
; Article
; chemical oxygen demand
; degradation
; desalination
; flocculation
; flotation
; fracking
; molecular weight
; ozonation
; priority journal
; waste water management
; waste water treatment plant
; adsorption
; chemistry
; metabolism
; procedures
; sewage
; waste water
; water pollutant
; Adsorption
; Carbon
; Charcoal
; Natural Gas
; Organic Chemicals
; Ozone
; Waste Disposal, Fluid
; Waste Water
; Water Pollutants, Chemical
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英文摘要: | Ozonation, sorption to granular activated carbon and aerobic degradation were compared as potential treatment methods for removal of dissolved organic carbon (DOC) fractions and selected organic compounds from shale gas flowback water after pre-treatment in dissolved air flotation unit. Flowback water was characterised by high chemical oxygen demand and DOC. Low molecular weight (LMW) acids and neutral compounds were the most abundant organic fractions, corresponding to 47% and 35% of DOC respectively. Ozonation did not change distribution of organic carbon fractions and concentrations of detected individual organic compounds significantly. Sorption to activated carbon targeted removal of individual organic compounds with molecular weight >115 Da, whereas LMW compounds remained largely unaffected. Aerobic degradation was responsible for removal of LMW compounds and partial ammonium removal, whereas formation of intermediates with molecular weight of 200–350 Da was observed. Combination of aerobic degradation for LMW organics removal with adsorption to activated carbon for removal of non-biodegradable organics is proposed to be implemented between pre-treatment (dissolved air floatation) and desalination (thermal or membrane desalination) steps. © 2018 Elsevier Ltd |
Citation statistics: |
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资源类型: | 期刊论文
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标识符: | http://119.78.100.158/handle/2HF3EXSE/112789
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Appears in Collections: | 气候减缓与适应
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作者单位: | Department of Environmental Technology, Wageningen University, P.O. Box 17, Wageningen, AA 6700, Netherlands; KWR Watercycle Research Institute, P.O. Box 1072, Nieuwegein, BB 3430, Netherlands; Copernicus Institute of Sustainable Development, Utrecht University, Heidelberglaan 2, Utrecht, 3584 CS, Netherlands
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Recommended Citation: |
Butkovskyi A.,Faber A.-H.,Wang Y.,et al. Removal of organic compounds from shale gas flowback water[J]. Water Research,2018-01-01,138
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