globalchange  > 气候减缓与适应
DOI: 10.1073/pnas.1812168116
WOS记录号: WOS:000455086900016
论文题名:
Anthropogenic drivers of 2013-2017 trends in summer surface ozone in China
作者: Li, Ke1,2; Jacob, Daniel J.2; Liao, Hong1,3; Shen, Lu2; Zhang, Qiang4; Bates, Kelvin H.2
通讯作者: Jacob, Daniel J. ; Liao, Hong
刊名: PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
ISSN: 0027-8424
出版年: 2019
卷: 116, 期:2, 页码:422-427
语种: 英语
英文关键词: surface ozone ; China ; aerosol chemistry ; emission reductions ; air quality
WOS关键词: CLIMATE-CHANGE ; SIGNIFICANT INCREASE ; PARTICULATE MATTER ; HAZE POLLUTION ; UNITED-STATES ; AIR-QUALITY ; SENSITIVITY ; EMISSIONS ; NORTH ; SITE
WOS学科分类: Multidisciplinary Sciences
WOS研究方向: Science & Technology - Other Topics
英文摘要:

Observations of surface ozone available from similar to 1,000 sites across China for the past 5 years (2013-2017) show severe summertime pollution and regionally variable trends. We resolve the effect of meteorological variability on the ozone trends by using a multiple linear regression model. The residual of this regression shows increasing ozone trends of 1-3 ppbv a(-1) in megacity clusters of eastern China that we attribute to changes in anthropogenic emissions. By contrast, ozone decreased in some areas of southern China. Anthropogenic NOx emissions in China are estimated to have decreased by 21% during 2013-2017, whereas volatile organic compounds (VOCs) emissions changed little. Decreasing NOx would increase ozone under the VOC-limited conditions thought to prevail in urban China while decreasing ozone under rural NOx-limited conditions. However, simulations with the Goddard Earth Observing System Chemical Transport Model (GEOS-Chem) indicate that a more important factor for ozone trends in the North China Plain is the similar to 40% decrease of fine particulate matter (PM2.5) over the 2013-2017 period, slowing down the aerosol sink of hydroperoxy (HO2) radicals and thus stimulating ozone production.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/127800
Appears in Collections:气候减缓与适应

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作者单位: 1.Nanjing Univ Informat Sci & Technol, Harvard NUIST Joint Lab Air Qual & Climate, Nanjing 210044, Jiangsu, Peoples R China
2.Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
3.Nanjing Univ Informat Sci & Technol, Sch Environm Sci & Engn, Collaborat Innovat Ctr Atmospher Environm & Equip, Jiangsu Key Lab Atmospher Environm Monitoring & P, Nanjing 210044, Jiangsu, Peoples R China
4.Tsinghua Univ, Dept Earth Syst Sci, Beijing 100084, Peoples R China

Recommended Citation:
Li, Ke,Jacob, Daniel J.,Liao, Hong,et al. Anthropogenic drivers of 2013-2017 trends in summer surface ozone in China[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2019-01-01,116(2):422-427
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