globalchange  > 气候变化事实与影响
DOI: 10.1016/j.envpol.2018.11.102
WOS记录号: WOS:000458222100039
论文题名:
Quantification of source specific black carbon scavenging using an aethalometer and a disdrometer
作者: Blanco-Alegre, C.1; Calvo, A. I.1; Coz, E.2; Castro, A.1; Oduber, F.1; Prevot, A. S. H.3; Mocnik, G.4; Fraile, R.1
通讯作者: Fraile, R.
刊名: ENVIRONMENTAL POLLUTION
ISSN: 0269-7491
EISSN: 1873-6424
出版年: 2019
卷: 246, 页码:336-345
语种: 英语
英文关键词: Black carbon ; BC scavenging estimation model ; Raindrop diameter ; Rainfall ; Scavenging coefficient ; Wet deposition
WOS关键词: CIRCULATION WEATHER TYPES ; AEROSOL-SIZE DISTRIBUTION ; AIR-POLLUTION ; PARTICULATE MATTER ; WET DEPOSITION ; URBAN ; CLIMATE ; PARTICLES ; PRECIPITATION ; HEALTH
WOS学科分类: Environmental Sciences
WOS研究方向: Environmental Sciences & Ecology
英文摘要:

Aerosol black carbon (BC) is the second strongest contributor to global warming, after CO2, and it is linked to many adverse health effects. A sampling campaign of 15 months was carried out in Leon (Spain) in order to evaluate the scavenging of BC with an ensemble aethalometer-disdrometer. The aethalometer provides the concentration of equivalent black carbon (eBC), and the disdrometer, the raindrop size distribution. A total of seventy-five rain events were studied and in 73% of them there was an effective (eBC(initial) > eBC(final)) scavenging, with a mean decrease of 48 +/- 37% in long rain events (>8 h) and 39 +/- 38% in short rain events. The scavenging of BC is strongly related to its source. Thus, the scavenging coefficient (SC) mean value of the BC from fossil fuel (eBC(ff)) for short and long rain events was 5.110(-5) and 1.3 10(-5) s(-1), respectively. For the BC from biomass burning (eBC(bb)), the SC values were 1.6 10(-4) and 2.8 10(-5) s(-1) in short and long events, respectively. There was a significant positive correlation between the SC and the number of drops with diameters between 0375 and 2.5 mm. Rain scavenging of eBC was analyzed depending on the air mass origin obtaining an effective scavenging for air masses from Atlantic, Arctic and Africa. A linear model (R-2 = 0.72) was built to estimate the Delta eBC values with variables from an aethalometer, a disdrometer and a weather station: eBC concentration before rain, swept volume and precipitation accumulated. A Kolmogorov-Smirnov statistical test confirmed the goodness of fit of the model to the measured data. (C) 2018 Elsevier Ltd. All rights reserved.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/130506
Appears in Collections:气候变化事实与影响

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作者单位: 1.IMARENAB Univ Leon, Dept Phys, Leon 24071, Spain
2.Ctr Energy Environm & Technol Res CIEMAT, Dept Environm, Madrid, Spain
3.Paul Scherrer Inst, Lab Atmospher Chem, CH-5232 Villigen, Switzerland
4.Jozef Stefan Inst, Dept Condensed Matter Phys, Ljubljana 1000, Slovenia

Recommended Citation:
Blanco-Alegre, C.,Calvo, A. I.,Coz, E.,et al. Quantification of source specific black carbon scavenging using an aethalometer and a disdrometer[J]. ENVIRONMENTAL POLLUTION,2019-01-01,246:336-345
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