globalchange  > 气候变化事实与影响
DOI: 10.1016/j.petrol.2018.12.034
WOS记录号: WOS:000458153000006
论文题名:
CO2/N-2 mixture sequestration in depleted natural gas hydrate reservoirs
作者: Zhou, Hang; Chen, Bingbing; Wang, Shenglong; Yang, Mingjun
通讯作者: Yang, Mingjun
刊名: JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING
ISSN: 0920-4105
EISSN: 1873-4715
出版年: 2019
卷: 175, 页码:72-82
语种: 英语
英文关键词: Carbon dioxide storage ; Gas hydrate ; Flue gas ; Natural gas hydrate reservoir
WOS关键词: CARBON-DIOXIDE SEPARATION ; METHANE HYDRATE ; FLUE-GAS ; THERMAL-STIMULATION ; CLATHRATE HYDRATE ; STORAGE CAPACITY ; POROUS-MEDIA ; CO2 CAPTURE ; FUEL GAS ; WATER
WOS学科分类: Energy & Fuels ; Engineering, Petroleum
WOS研究方向: Energy & Fuels ; Engineering
英文摘要:

Carbon dioxide (CO2) emission is one of the primary causes of global warming, while CO2 storage is an effective way to solve this problem. Moreover, CO2 storage as CO2 hydrate is regarded as a viable and promising way. The development of natural gas hydrate mining technologies has provided a safe and appropriate method to store CO2 in depleted gas hydrate reservoirs. In addition, different concentrations of N-2 are contained in the captured CO2 from flue gas. Therefore, CO2 storage with different N-2 concentrations in depleted natural gas hydrate reservoirs with excess water was investigated in this study. Three types of gas (pure CO2, 90 mol%CO2 + 10 mol %N-2 and 80 mol%CO2 + 20 mol%N-2) and three pressures (3.0 MPa, 3.2 MPa and 3.5 MPa) in the constant pressure process were investigated. Magnetic Resonance Imaging (MRI) was employed to monitor the entire experimental process. The experimental results showed that the hydrate was nucleated and generated in different areas independently during the storage process. N-2 was beneficial for quick hydrate formation; however, pure CO2 was most efficient for hydrate formation from a long-term perspective. In addition, CO2 was primarily stored as hydrate; a portion of CO2 was stored in the form of gas; and a small amount of CO2 was dissolved in the pore water. Moreover, the CO2 storage density (226.56 kg/m(3)) was the highest at the conditions of 275.15 K and 3.5 MPa using 90 mol%CO2 + 10 mol%N-2 in the experiments. The highest CO2 storage density (229.99 kg/m(3)) calculated through water conversion occurred at the conditions of 275.15 K and 3.5 MPa using pure CO2.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/133020
Appears in Collections:气候变化事实与影响

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作者单位: Dalian Univ Technol, Minist Educ, Key Lab Ocean Energy Utilizat & Energy Conservat, Dalian 116024, Liaoning, Peoples R China

Recommended Citation:
Zhou, Hang,Chen, Bingbing,Wang, Shenglong,et al. CO2/N-2 mixture sequestration in depleted natural gas hydrate reservoirs[J]. JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING,2019-01-01,175:72-82
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