globalchange  > 气候变化事实与影响
DOI: 10.1080/02786826.2019.1599320
WOS记录号: WOS:000466682000001
论文题名:
Models for the bead mobility technique: A droplet-based viscometer
作者: Sellier, M.1; Taylor, J.1; Bertram, A. K.2; Mandin, P.3
通讯作者: Sellier, M.
刊名: AEROSOL SCIENCE AND TECHNOLOGY
ISSN: 0278-6826
EISSN: 1521-7388
出版年: 2019
卷: 53, 期:7, 页码:749-759
语种: 英语
WOS关键词: SECONDARY ORGANIC MATERIAL ; SHEAR-FLOW ; SMALL VOLUMES ; VISCOSITIES ; CIRCULATION ; GROWTH ; FLUID ; STATE ; WALL
WOS学科分类: Engineering, Chemical ; Engineering, Mechanical ; Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向: Engineering ; Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
英文摘要:

Better understanding the properties of organic aerosols (OA) is attracting increasing attention because of the important role they play in climate change. The viscosity of OA has been shown to range from liquid to solid/semi-solid across the range of atmospheric relative humidity. A method known as the "bead-mobility technique" has been developed to quantify the viscosity of an atmospheric particle over a range of atmospherically relevant humidities. The method is based on the assumption that the strength of the flow recirculation inside a droplet placed in a shear flow is related to the droplet viscosity. This article presents a simple analytical model which predicts the internal flow in the droplet and provides a correlation relating the strength of the flow in the droplet to its viscosity. The validity of this analytical model is assessed by comparing the analytical results with a corresponding two-phase flow simulation with a moving mesh which captures the motion of the interface. The ability of the analytical model to reproduce experimental data reported in the literature is also quantified. The reasonable agreement between the analytical model and the experimental data confirms that the droplet velocity provides a useful proxy to estimate the droplet viscosity for small liquid samples for which standard viscometry techniques do not apply. Copyright (c) 2019 American Association for Aerosol Research


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/134260
Appears in Collections:气候变化事实与影响

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作者单位: 1.Univ Canterbury, Dept Mech Engn, Private Bag 4800, Christchurch 8140, New Zealand
2.Univ British Columbia, Dept Chem, Vancouver, BC, Canada
3.Univ Bretagne Sud, IRDL, UMR CNRS 6027, Lorient, France

Recommended Citation:
Sellier, M.,Taylor, J.,Bertram, A. K.,et al. Models for the bead mobility technique: A droplet-based viscometer[J]. AEROSOL SCIENCE AND TECHNOLOGY,2019-01-01,53(7):749-759
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