globalchange  > 过去全球变化的重建
DOI: 10.1029/2018GL081731
WOS记录号: WOS:000468869500048
论文题名:
Long-Term Measurements Show Little Evidence for Large Increases in Total US Methane Emissions Over the Past Decade
作者: Lan, Xin1,2; Tans, Pieter2; Sweeney, Colm2; Andrews, Arlyn2; Dlugokencky, Edward2; Schwietzke, Stefan1,2; Kofler, Jonathan1,2; McKain, Kathryn1,2; Thoning, Kirk2; Crotwell, Molly1,2; Montzka, Stephen2; Miller, Benjamin R.1,2; Biraud, Sebastien C.3
通讯作者: Lan, Xin
刊名: GEOPHYSICAL RESEARCH LETTERS
ISSN: 0094-8276
EISSN: 1944-8007
出版年: 2019
卷: 46, 期:9, 页码:4991-4999
语种: 英语
WOS关键词: NATURAL-GAS PRODUCTION ; TROPOSPHERIC DISTRIBUTION ; NONMETHANE HYDROCARBONS ; NORTH-AMERICA ; FOSSIL-FUEL ; ETHANE ; OIL ; SCALE ; CO2 ; BUDGET
WOS学科分类: Geosciences, Multidisciplinary
WOS研究方向: Geology
英文摘要:

Recent studies show conflicting estimates of trends in methane (CH4) emissions from oil and natural gas (ONG) operations in the United States. We analyze atmospheric CH4 measurements from 20 North American sites in the National Oceanic and Atmospheric Administration Global Greenhouse Gas Reference Network and determined trends for 2006-2015. Using CH4 vertical gradients as an indicator of regional surface emissions, we find no significant increase in emissions at most sites and modest increases at three sites heavily influenced by ONG activities. Our estimated increases in North American ONG CH4 emissions (on average approximately 3.4 +/- 1.4 %/year for 2006-2015, +/-sigma) are much smaller than estimates from some previous studies and below our detection threshold for total emissions increases at the east coast sites that are sensitive to U.S. outflows. We also find an increasing trend in ethane/methane emission ratios, which has resulted in major overestimation of oil and gas emissions trends in some previous studies.


Plain Language Summary In the past decade, natural gas production in the United States has increased by similar to 46%. Methane emissions associated with oil and natural gas productions have raised concerns since methane is a potent greenhouse gas with the second largest influence on global warming. Recent studies show conflicting results regarding whether methane emissions from oil and gas operations have been increased in the United States. Based on long-term and well-calibrated measurements, we find that (i) there is no large increase of total methane emissions in the United States in the past decade; (ii) there is a modest increase in oil and gas methane emissions, but this increase is much lower than some previous studies suggest; and (iii) the assumption of a time-constant relationship between methane and ethane emissions has resulted in major overestimation of an oil and gas emissions trend in some previous studies.


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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/138447
Appears in Collections:过去全球变化的重建

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作者单位: 1.Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
2.NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA
3.Lawrence Berkeley Nat Lab, Berkeley, CA USA

Recommended Citation:
Lan, Xin,Tans, Pieter,Sweeney, Colm,et al. Long-Term Measurements Show Little Evidence for Large Increases in Total US Methane Emissions Over the Past Decade[J]. GEOPHYSICAL RESEARCH LETTERS,2019-01-01,46(9):4991-4999
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