globalchange  > 全球变化的国际研究计划
DOI: 10.1002/ese3.334
WOS记录号: WOS:000479313100007
论文题名:
Effect of internal hydrocarbon reforming during coupled operation of a biomass gasifier with hot gas cleaning and SOFC stacks
作者: Fischer, Felix1; Hauser, Michael1; Hauck, Maximilian1; Herrmann, Stephan1; Fendt, Sebastian1; Jeong, Hyeondeok2; Lenser, Christian2; Menzler, Norbert H.2; Spliethoff, Hartmut1,3
通讯作者: Fischer, Felix
刊名: ENERGY SCIENCE & ENGINEERING
ISSN: 2050-0505
出版年: 2019
卷: 7, 期:4, 页码:1140-1153
语种: 英语
英文关键词: biomass gasification ; bio-syngas ; solid oxide fuel cells ; tar reforming
WOS关键词: OXIDE FUEL-CELL ; STEAM-GASIFICATION ; CARBON FORMATION ; FLUIDIZED-BED ; TAR ; SYNGAS ; DEGRADATION ; PERFORMANCE ; ANODE ; PHENOL
WOS学科分类: Energy & Fuels
WOS研究方向: Energy & Fuels
英文摘要:

In the context of energy transition and climate change, a combination of highly efficient modern solid oxide fuel cells (SOFC) and thermo-chemical conversion of biogenic residues could complement other intermittent renewable sources such as wind and solar. In order to reduce required gas cleaning efforts and to increase the process efficiency, the influence of hydrocarbons on SOFC performance is experimentally investigated in this study. For the first time, the operation of Ni/YSZ anode-supported cells in Julich F10 stacks is performed with pre-reformed and with bio-syngas containing full hydrocarbon content at realistic current densities. Sulfur and other impurities were removed in both cases. No degradation could be observed within normal operation on clean gas. With the tar reformer bypassed, the pressure drop over the stack increased due to severe carbon deposition on the anode substrate and the nickel current collector mesh inside the SOFC stack, so that operation had to be terminated after five hours. This behavior is different from single-cell tests, where electrochemical degradation is the limiting factor. The results show that improvements are not only necessary for cell materials and that future research must also consider other stack components.


Citation statistics:
被引频次[WOS]:9   [查看WOS记录]     [查看WOS中相关记录]
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/144577
Appears in Collections:全球变化的国际研究计划

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作者单位: 1.Tech Univ Munich, Chair Energy Syst, Garching, Germany
2.Forschungszentrum Julich, Julich, Germany
3.Bayer Zentrum Angew Energieforsch eV, Garching, Germany

Recommended Citation:
Fischer, Felix,Hauser, Michael,Hauck, Maximilian,et al. Effect of internal hydrocarbon reforming during coupled operation of a biomass gasifier with hot gas cleaning and SOFC stacks[J]. ENERGY SCIENCE & ENGINEERING,2019-01-01,7(4):1140-1153
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