globalchange  > 气候变化事实与影响
CSCD记录号: CSCD:6291243
论文题名:
环保型绝缘介质C_5F_(10)O放电分解特性
其他题名: Study on the Discharge Decomposition Characteristics of an Environmental-friendly Insulating Medium C_5F_(10)O
作者: 李祎1; 张晓星1; 肖淞1; 黄立群2; 唐炬1; 邓载韬1; 田双双1
刊名: 中国电机工程学报
ISSN: 0258-8013
出版年: 2018
卷: 38, 期:14, 页码:744-752
语种: 中文
中文关键词: C_5F_(10)O分解特性 ; 环保型绝缘介质 ; 密度泛函理论 ; 前线分子轨道理论 ; 能量变化
英文关键词: C_5F_(10)O decomposition characteristics ; environmental-friendly insulating medium ; density functional theory ; frontier molecular orbital theory ; energy change
WOS学科分类: ENGINEERING ELECTRICAL ELECTRONIC
WOS研究方向: Engineering
中文摘要: 近期,CnF_2nO类物质得到了替代气体研究领域的关注,尤其是C_5F_(10)O和C_6F_(12)O,两者均具有极低的温室效应潜能指数(global warming potential,GWP)且绝缘特性优异。由于其出色的绝缘表现,国内外科研机构和公司开始关注该物质及其混合气体,目前针对其放电分解特性的研究较少。该文基于密度泛函理论从微观层面对C_5F_(10)O的稳定性及可能的分解路径展开分析,首先计算得到C_5F_(10)O的电离能等参数,并基于前线分子轨道理论确定分子结构中可能发生反应的位置。其次,分析C_5F_(10)O可能的分解途径、分解产物的形成机制并计算得到相应的能量变化。最后,利用气体绝缘试验平台对C_5F_(10)O/N_2混合气体进行击穿测试,基于气相色谱质谱联用仪对击穿前后气室内气体组分进行分析,探讨分解产物的绝缘性能及放电过程中各类粒子的动态平衡过程。研究结果表明,C_5F_(10)O放电分解形成CF_3CO·、C_3F_7·或C_3F_7CO·、CF_3·自由基的过程最容易发生,各类自由基进一步反应将生成CF_4、C_2F_6、C_3F_8、C_3F_6、C_4F_(10)、C_5F_(12)、 C_6F_(14),上述产物均具有较强的绝缘性能,且C_5F_(10)O分子与自由基间存在动态平衡过程,两者共同保障了体系的绝缘性能。试验发现随着击穿次数的增加,C_5F_(10)O各分解产物含量增加,其中CF_4、C_2F_6、C_4F_(10)的增长率高于C_3F_8、C_6F_(14),自由基更易于复合形成小分子产物。相关结论对进一步探究C_5F_(10)O混合气体的绝缘特性及协同效应等课题提供一定理论依据,同时为CnF_2nO类新型环保型介质研究提供一些借鉴。
英文摘要: Recently,the CnF_2nO species have received much attention in the field of alternative gases,particularly C_5F_(10)O and C_6F_(12)O,both of which have a very low global warming potential(GWP)and excellent insulation properties.Due to its excellent insulation performance,foreign scientific research institutions and companies begin to study the material and its mixture,and there are few studies on its decomposition characteristics under discharge.In this paper,based on the density functional theory,the stability of C_5F_(10)O and its possible decomposition path were analyzed.At first,the ionization energy of C_5F_(10)O was calculated,and the possible position of the reaction in the molecular structure was determined based on the frontier molecular orbital theory.Secondly,the possible decomposition pathway of C_5F_(10)O,the formation mechanism of the decomposition products and the corresponding energy changes were analyzed.Finally,the C_5F_(10)O/N_2 gas mixture was tested by using gas insulated test platform,the gas components in the gas chamber before and after breakdown were analyzed based on gas chromatography mass spectrometry(GC-MS),the insulation properties of the decomposition products and the dynamic equilibrium processes of various particles during the discharge process were discussed.The results show that the formation of CF_3CO·,C_3F_7·or C_3F_7CO·,CF_3·radicals is most likely to occur during the decomposition of C_5F_(10)O,and further reactions of various free radicals will generate CF_4,C_2F_6,C_3F_8,C_3F_6,C_4F_(10),C_5F_(12),C_6F_(14).The products have strong insulating properties,and the dynamic equilibrium between C_5F_(10)O molecules and free radicals exists,both of which ensure the insulation performance of the system.The test results showed that with the increase of breakdown times,the content of C_5F_(10)O decomposition products increased,and the growth rate of CF_4,C_2F_6 and C_4F_(10) was higher than that of C_3F_8 and C_6F_(14).The conclusions provide theoretical basis for further research of insulation properties and synergistic effect of C_5F_(10)O gas mixture,and provide a reference for the study of CnF_2nO environmentalfriendly medium.
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/155218
Appears in Collections:气候变化事实与影响

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作者单位: 1.武汉大学电气工程学院, 武汉, 湖北 430072, 中国
2.ABB(中国)有限公司, 厦门, 福建 361006, 中国

Recommended Citation:
李祎,张晓星,肖淞,等. 环保型绝缘介质C_5F_(10)O放电分解特性[J]. 中国电机工程学报,2018-01-01,38(14):744-752
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