globalchange  > 气候变化与战略
DOI: 10.1016/j.atmosenv.2019.117201
论文题名:
Aerosol radiative impact on surface ozone during a heavy dust and biomass burning event over South Asia
作者: Mukherjee T.; Vinoj V.; Midya S.K.; Adhikary B.
刊名: Atmospheric Environment
ISSN: 1352-2310
出版年: 2020
卷: 223
语种: 英语
英文关键词: Aerosols ; Air quality ; Atmospheric movements ; Boundary layer flow ; Boundary layers ; Budget control ; Dust ; Ozone ; Photolysis ; Black carbon ; Boundary layer heights ; Chemical transport models ; Emission inventories ; Meteorological parameters ; Photolysis frequencies ; Surface ozone concentrations ; WRF-Chem ; Ozone layer ; black carbon ; ozone ; aerosol composition ; air quality ; biomass burning ; black carbon ; concentration (composition) ; heavy metal ; ozone ; radiative forcing ; aerosol ; air quality ; biomass ; dust ; fire ; meteorology ; model ; photolysis ; priority journal ; radiation ; South Asia
学科: Black carbon ; Dust ; Ozone ; Radiative feedback ; WRF-Chem
中文摘要: Aerosols can modify both short and long term weather patterns by impacting the radiation budget of Earth. Numerical simulations were performed to understand the direct effect of aerosol on radiation during an elevated dust and black carbon (BC) concentration period over south Asia. The impact of the aerosol (dust and BC separately) direct effect on meteorology and air quality (focusing on surface ozone) was assessed using a fully coupled chemical transport model (WRF-Chem). The model simulates the elevated dust and BC concentration plume well qualitatively. Our results show that elevated BC concentration can reduce surface temperature up to 2 K. Incoming short wave flux at the surface and the boundary layer height reduced up to 70% due to the radiative impact of BC. ‘This reduction in boundary layer height further increases the BC concentration at the source region. The radiative impact of dust on meteorological parameters are found to be less compared to BC at the surface level. The model simulates realistic surface ozone concentration using HTAP emission inventory. Results reveal that the presence of biomass burning can increase the surface ozone concentration by up to 40%. The radiative impact of BC can reduce the surface ozone concentration by more than 30% by altering the photolysis frequencies. © 2020 Elsevier Ltd
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/160577
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作者单位: International Centre for Integrated Mountain Development, Nepal; School of Earth, Ocean and Climate Sciences, Indian Institute of Technology, Bhubaneswar, India; Department of Atmospheric Science, University of Calcutta, India

Recommended Citation:
Mukherjee T.,Vinoj V.,Midya S.K.,et al. Aerosol radiative impact on surface ozone during a heavy dust and biomass burning event over South Asia[J]. Atmospheric Environment,2020-01-01,223
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