globalchange  > 气候变化与战略
DOI: 10.1016/j.scib.2019.12.009
论文题名:
Coherent and incoherent theories for photosynthetic energy transfer
作者: Tao M.-J.; Zhang N.-N.; Wen P.-Y.; Deng F.-G.; Ai Q.; Long G.-L.
刊名: Science Bulletin
ISSN: 20959273
出版年: 2020
卷: 65, 期:4
起始页码: 318
结束页码: 328
语种: 英语
中文关键词: Coherent modified Redfield theory ; Förster theory ; General Bloch-Redfield theory ; Hierarchical equation of motion ; Modified Redfield theory ; Small-polaron quantum master equation
英文关键词: Energy transfer ; Equations of motion ; Polarons ; Quantum chemistry ; Quantum theory ; Artificial light harvesting ; Bloch-Redfield theory ; Energy transfer efficiency ; Equation of motion ; Experimental techniques ; Quantum coherent effects ; Quantum master equations ; Redfield theory ; Artificial photosynthesis
英文摘要: There is a remarkable characteristic of photosynthesis in nature, that is, the energy transfer efficiency is close to 100%. Recently, due to the rapid progress made in the experimental techniques, quantum coherent effects have been experimentally demonstrated. Traditionally, the incoherent theories are capable of calculating the energy transfer efficiency, e.g., (generalized) Förster theory and modified Redfield theory (MRT). However, in order to describe the quantum coherent effects in photosynthesis, one has to exploit coherent theories, such as hierarchical equation of motion (HEOM), quantum path integral, coherent modified Redfield theory (CMRT), small-polaron quantum master equation, and general Bloch-Redfield theory in addition to the Redfield theory. Here, we summarize the main points of the above approaches, which might be beneficial to the quantum simulation of quantum dynamics of exciton energy transfer (EET) in natural photosynthesis, and shed light on the design of artificial light-harvesting devices. © 2019 Science China Press
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/170049
Appears in Collections:气候变化与战略

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作者单位: Department of Physics, Tsinghua University, Beijing, 100084, China; Department of Physics, Applied Optics Beijing Area Major Laboratory, Beijing Normal University, Beijing, 100875, China; NAAM-Research Group, Department of Mathematics, Faculty of Science, King Abdulaziz University, Jeddah, 21589, Saudi Arabia

Recommended Citation:
Tao M.-J.,Zhang N.-N.,Wen P.-Y.,et al. Coherent and incoherent theories for photosynthetic energy transfer[J]. Science Bulletin,2020-01-01,65(4)
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