globalchange  > 气候变化事实与影响
DOI: doi:10.1038/nclimate2727
论文题名:
The possible role of local air pollution in climate change in West Africa
作者: Peter Knippertz
刊名: Nature Climate Change
ISSN: 1758-788X
EISSN: 1758-6908
出版年: 2015-08-21
卷: Volume:5, 页码:Pages:815;822 (2015)
语种: 英语
英文关键词: Atmospheric chemistry
英文摘要:

The climate of West Africa is characterized by a sensitive monsoon system that is associated with marked natural precipitation variability. This region has been and is projected to be subject to substantial global and regional-scale changes including greenhouse-gas-induced warming and sea-level rise, land-use and land-cover change, and substantial biomass burning. We argue that more attention should be paid to rapidly increasing air pollution over the explosively growing cities of West Africa, as experiences from other regions suggest that this can alter regional climate through the influences of aerosols on clouds and radiation, and will also affect human health and food security. We need better observations and models to quantify the magnitude and characteristics of these impacts.

The West African monsoon is one of the most important large-scale atmospheric circulation systems in the tropics. It controls winds, temperature, clouds and most importantly precipitation over a land area of about 6 × 106 km2 (~5–25° N, 15° W to 15° E) and has remote impacts, for example through hurricane genesis. Through water resources, agriculture and power generation, the health and livelihoods of hundreds of millions of people depend on monsoonal rainfall.

The West African monsoon is a sensitive system that can be perturbed by different factors across a wide range of scales. A prominent example is the devastating drought in the 1970s and 1980s1 that most severely affected the Sahel, one of the regions with the largest precipitation variability worldwide. A large fraction of decadal-scale rainfall variability in the West African monsoon area is explained by variations in Atlantic sea-surface temperatures, which have been linked to natural oscillations but also to changes in anthopogenic aerosol emissions during the twentieth century, predominantly from industrialized areas in the mid-latitudes2, 3. It is anticipated that the West Africa regional climate will change because of the effects of global-scale warming, implying an increased likelihood of unprecedented heat waves and a threat to low-lying, densely populated coastal areas from sea-level rise4, and also because of land-use and land-cover change, as the increasing transformation of rain and savannah forests into agricultural land creates changes in the surface energy and water balance through effects on albedo, evapotranspiration, water transport and storage as well as surface roughness5, 6.

Studies on the Indian and East Asian monsoons suggest that anthropogenic emissions of aerosols and aerosol precursor gases from these densely populated and increasingly industrialized areas can affect the amount and seasonality of rainfall. Earlier studies concentrated on scattering aerosols such as sulphates, which reduce monsoonal circulation and precipitation through a reduction of short-wave radiation reaching the surface, sometimes termed 'solar dimming'7. The inclusion of absorbing aerosols such as black carbon creates a more complicated response in models that, among other things, depends on whether a coupling to the ocean is taken into account8. According to the 'elevated heat pump' concept, aerosol heating over the Tibetan Plateau causes large-scale circulation changes over South and East Asia9, but this idea is difficult to prove from observations10. Recent studies are increasingly including effects of aerosols on clouds and typically find a reduction of monsoon-season precipitation through the combined effects of clouds and radiation changes11, 12.

In West Africa anthropogenic emissions of aerosols and aerosol precursor gases have increased rapidly in recent years and are projected to keep increasing13, 14. This is particularly the case for the explosively growing cities along the Guinea Coast, as illustrated by high aerosol optical thickness along the coastal strip in the satellite image shown in Fig. 1, particularly in the area of Lagos. In this Perspective we will discuss the question of whether this increasing pollution can be expected to perturb the sensitive West African monsoon system and thereby contribute to regional climate change in addition to the more established long-term factors global warming and regional land-use and land-cover change. In contrast to the Indian and East Asian monsoon, this emerging research topic has not received much attention and therefore the relative magnitude of this problem and possible interactions of different factors are unclear. Undoubtedly urban air pollution has already become a significant threat for human and ecosystem health across West African cities such that any regulatory actions could have multiple benefits. We will begin with a short overview of the meteorological conditions over West Africa followed by a discussion of anthropogenic aerosols and aerosol-climate interactions. Concrete steps needed to improve our understanding of the role of air pollution for the West African climate are given in the concluding section.

Figure 1: Sea breeze, clouds and pollution.
Sea breeze, clouds and pollution.

MODIS visible image at 13:35 UTC on 12 October 2013 over southern West Africa showing a well-defined land–sea breeze and small-scale cumulus inland. MODIS aerosol optical depth at 0.55 μm wavelength is overlaid as colour shading in areas where the retrieval algorithm96 determines the image to be sufficiently cloud-free. This product shows enhanced air pollution along the coast and over the Gulf of Guinea, particularly in the vicinity of the coastal cities marked.

The West African monsoon is associated with a marked seasonal cycle. From November to February most of the region is dominated by dry northeasterly winds from the Sahara. Clouds and precipitation are confined to the coastal strip, where the sea-breeze circulation brings in moister air and creates near-surface convergence. Large amounts of mineral dust from the Sahel and Sahara are transported across the region, which in combination with human-induced biomass burning lead to persistent haze because of the lack of wet removal. From March onwards the southwesterly monsoon winds begin to penetrate deeper into the continent, bringing with them moister air, more clouds and precipitation15. The monsoon retreats back to the southern parts of West Africa in September and October. At the peak of the wet season in July and August, the large meridional low-level pressure gradient between the cold sea-surface temperatures in the eastern equatorial Atlantic Ocean and the Saharan heat low drives a strong monsoon flow with southwesterlies reaching about 20° N (Fig. 2a). The reduction in turbulence and therefore depth of the frictional layer from day to night leads to the formation of strong nocturnal low-level jets16, 17, 18 (Fig. 2b) that transport moist air far into the continent.

Figure 2: Clouds and the West African monsoon.
Clouds and the West African monsoon.

a, Schematic meridional-pressure section illustrating the West African monsoon circulation, main cloud types (dark grey for frequent and light grey for less frequent occurrence), moist monsoonal layer characterized by southwesterly winds (red shading) and the African easterly jet (AEJ, blue shading). Grey lines are isentropic surfaces; the 0 °C isotherm is marked. b, Zoom into the processes involved in the formation and maintenance of low-level stratus decks over southern West Africa. Vectors show a typical vertical profile of horizontal wind; NLLJ indicates the nocturnal low-level jet. This figure is derived from high-resolution modelling28. Panel b reproduced with permission from ref. 28, AMS.

Much of our current understanding of the regional atmospheric composition over West Africa stems from the African Monsoon Multidisciplinary Analysis (AMMA)30 project31 and other activities such as the DECAFE (Dynamique et Chimie Atmosphérique en Forêt Equatoriale) programme, the IGAC (International Global Atmospheric Chemistry)/DEBITS (Deposition of Biogeochemically Important Trace Species)/AFRICA atmospheric chemistry and deposition monitoring network IDAF (http://idaf.sedoo.fr; in operation since 1995) and the Aerosol Robotic Network (AERONET)32. The bulk of this work, though, focused on the substantial natural emissions from deserts, soils, forests and oceans, and thus on more remote parts of the region. This pertains to both observations and modelling.

In West Africa, biomass burning is a large direct source of carbonaceous aerosols, which have a strong radiative effect, and also of volatile organic compounds, oxides of nitrogen, carbon monoxide and so on, which can indirectly impact climate through perturbing ozone and methane concentrations and through creating secondary aerosol particles. Biomass burning occurs predominantly during the dry season. It is almost exclusively anthropogenic following century-old traditional practices31, 33.

An additional factor that has received surprisingly little attention thus far is anthropogenic emissions of domestic, traffic and industrial pollutants. Although the increase of the global population is slowing down, the population of West Africa continues to increase by 2–3% per year (Fig. 3), with the current population of around 340 million projected to reach more than 800 million by the middle of the century34. This increase is accompanied by strong economic growth of currently about 5% per year, as well as industrialization and rapid urbanization (Fig. 3). As a result, pollutants such as oxides of nitrogen and sulphur, hydrocarbons, carbon monoxide and carbonaceous aerosols have increased sharply over the past decades and, depending on compound and scenario, are projected to increase between two- and fourfold by 2030 (Fig. 4a). They would then contribute between about 5 and 60% of global emissions, depending on compound and scenario13, 14. A significant source of uncertainty in these predictions lies in the degree of regulatory constraint on emissions anticipated by the different West African countries over these decades.

Figure 3: Trends in West African population and settlement patterns.
Trends in West African population and settlement patterns.

Dashed black line: estimates and growth projections of the region's total population between 1950 and 2020 (ECOWAS member states plus Mauritania) taken from United Nations (UN) data. Red line: urban population according to the Africapolis study based on analysis of satellite/ aerial images and census data. Figures in italics indicate average annual increase for that decade. Green line: rural population according to official estimates. Solid black line: sum of red and green lines, showing possible disagreement with UN estimates. Grey lines give ratios of urban to rural (U/R) population for the two different estimates. Note semi-logarithmic scale. Figure adapted with permission from ref. 97, SWAC/OECD.

Generally, aerosols affect climate through impacts on radiation and clouds. The physical understanding of direct radiative effects is comparatively good, but uncertainties are introduced through insufficient knowledge of the vertical distribution and optical properties of the particles that depend on size distribution, shape and chemical composition, whereas interactions between aerosols and clouds are less well understood — particularly for ice and mixed-phase clouds54, 55 — and remain one of the most uncertain anthropogenic forcings of the Earth's climate56.

For West Africa, most of the aerosol–climate interaction studies look at radiative effects of dust and biomass burning aerosols. Black carbon from man-made fires during the dry season has been suggested to reduce precipitation in West Africa by changing the atmospheric circulation, leading to reductions of cloud frequencies and height57. Similar impacts have been found from the radiative effects of desert dust58, 59. Urban pollution can enhance downwelling radiation during clear nights and therefore cause large increases in night-time minimum temperatures as warm air is mixed from aloft because of radiative destabilization60, but this has not been investigated for the Guinea Coastal zone, where additional impacts on the nocturnal low-level jet and stratus formation can be expected26, 28.

To the best of our knowledge, there are no studies looking into aerosol–cloud interactions over the moister southern parts of West Africa. This is partly due to a sparse network of measurements for atmospheric composition and meteorological variables61 and partly due to the historically low levels of industrial development. Aerosols directly affect the properties of cloud droplets and ice crystals, which then in turn affect cloud-top height, albedo, areal extent and lifetime, and the cloud's environment; that is, there are two-way couplings between the cloud's microphysical and macrophysical properties62, 63, 64, 65, 66. As a result, the effects of aerosols on single clouds can be very different from when a system of clouds evolving through many cloud lifetimes is considered. Such aerosol effects have barely been considered for the meteorological environment of the West African monsoon.

Previous research in regions affected by biomass burning67 has shown that the size distribution and number concentration of the aerosol particles are the main predictor of the concentration of cloud condensation nuclei (CCN), whereas composition and hygroscopicity are less important. However, secondary organic aerosols may play a role in complicating predictions of CCN concentration68. Studies on the extensive marine stratus decks in subtropical high-pressure regions show that an increase in aerosols can lead to changes of up to 40% of the reflected shortwave radiation69 and can inhibit rainfall, with lightly precipitating clouds affected most severely70. In summertime West Africa, the nocturnal low-level jet carries pollution from the coastal belt inland, where interactions with biogenic emissions from fields and forests may lead to the formation of secondary aerosol particles as discussed above. These aerosols are likely to be mixed into the extensive low stratus decks over the region (see Fig. 2). It would therefore be interesting to investigate possible changes to the clouds' radiative effects71, which in turn could change the evolution of the boundary layer and consequently the diurnal cycle of convection72. Changes to the areal cover, longevity or brightness of the West African stratus clouds could then have an effect on surface radiation due to the albedo contrast with the underlying dark forest areas27. This may ultimately affect larger parts of the West African monsoon system through changes to the regional circulation. Unfortunately, current climate models seem to struggle with realistically representing both low- and mid-level clouds in this region, resulting in a spread of up to 90 W m−2 in the regional mean daily surface solar irradiance27, 73. Couvreux et al.74 show that the cloud radiative errors are already established after a few days' simulation time and seem to be related to the complex local energy balances and boundary-layer processes rather than large-scale advection18. These errors may therefore be related to problems with the model parameterizations of convection and the boundary layer, demonstrating the challenge of realistically representing cloud–aerosol effects in this region in models.

For convective clouds, modelling studies have shown that aerosol effects are typically more important in situations with relatively low convective available potential energy75, as is often the case along the Guinea Coast. Detailed mechanisms have been proposed for single clouds, such as the concept of convective invigoration63 that links increased aerosol loading to deeper, more vigorous convection by chaining together a number of physical processes. However, breaks in that chain or differences introduced by considering additional physical process

URL: http://www.nature.com/nclimate/journal/v5/n9/full/nclimate2727.html
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/4616
Appears in Collections:气候变化事实与影响
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Peter Knippertz. The possible role of local air pollution in climate change in West Africa[J]. Nature Climate Change,2015-08-21,Volume:5:Pages:815;822 (2015).
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