DOI: 10.5194/cp-9-243-2013
Scopus记录号: 2-s2.0-84873889475
论文题名: A biomarker record of Lake El'gygytgyn, Far East Russian arctic: Investigating sources of organic matter and carbon cycling during marine isotope stages 1-3
作者: Holland A.R. ; Petsch S.T. ; Castañeda I.S. ; Wilkie K.M. ; Burns S.J. ; Brigham-Grette J.
刊名: Climate of the Past
ISSN: 18149324
出版年: 2013
卷: 9, 期: 1 起始页码: 243
结束页码: 260
语种: 英语
Scopus关键词: anoxic conditions
; biomarker
; carbon cycle
; carbon isotope
; climate change
; glaciation
; isotopic analysis
; isotopic composition
; lacustrine deposit
; Last Glacial Maximum
; marine environment
; organic carbon
; organic matter
; paleoenvironment
; sediment chemistry
; water column
; Chukchi
; Elgygytgyn Lake
; Russian Federation
英文摘要: Arctic paleoenvironmental archives serve as sensitive recorders of past climate change. Lake El'gygytgyn (Far East Russian Arctic) is a high-latitude crater impact lake that contains a continuous sediment record influenced by neither glaciation nor glacial erosion since the time of impact 3.58 Ma ago. Prior research on sediments collected from Lake El'gygytgyn suggest times of permanent ice cover and anoxia corresponding to global glacial intervals, during which the sediments are laminated and are characterized by the co-occurrence of high total organic carbon, microscopic magnetite grains that show etching and dissolution, and negative excursions in bulk sediment organic matter carbon isotope (δ13C) values. Here we investigate the abundance and carbon isotopic composition of lipid biomarkers recovered from Lake El'gygytgyn sediments spanning marine isotope stages 1-3 to identify key sources of organic matter (OM) to lake sediments, to establish which OM sources drive the negative δ13C excursion exhibited by bulk sediment OM, and to explore if there are molecular and isotopic signatures of anoxia in the lake during glaciation. We find that during marine isotope stages 1-3, direct evidence for water column anoxia is lacking. A ∼4‰ negative excursion in bulk sediment δ13C values during the Local Last Glacial Maximum (LLGM) is accompanied by more protracted, higher magnitude negative excursions in n-alkanoic acid and n-alkanol δ13C values that begin 20 kyr in advance of the LLGM. In contrast, n-alkanes and the C30 n-alkanoic acid do not exhibit a negative δ13C excursion at this time. Our results indicate that the C24, C26 and C28 n-alkanoic acids do not derive entirely from terrestrial OM sources, while the C30 n-alkanoic acid at Lake El'gygytgyn is a robust indicator of terrestrial OM contributions. Overall, our results strongly support the presence of a nutrient-poor water column, which is mostly isolated from atmospheric carbon dioxide during glaciation at Lake El'gygytgyn. © 2013 Author(s). Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/49472
Appears in Collections: 气候变化与战略
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Recommended Citation:
Holland A.R.,Petsch S.T.,Castañeda I.S.,et al. A biomarker record of Lake El'gygytgyn, Far East Russian arctic: Investigating sources of organic matter and carbon cycling during marine isotope stages 1-3[J]. Climate of the Past,2013-01-01,9(1)