globalchange  > 气候变化事实与影响
DOI: 10.5194/hess-21-5725-2017
Scopus记录号: 2-s2.0-85034600069
论文题名:
Impact of snow deposition on major and trace element concentrations and elementary fluxes in surface waters of the Western Siberian Lowland across a 1700'km latitudinal gradient
作者: Shevchenko V; P; , Pokrovsky O; S; , Vorobyev S; N; , Krickov I; V; , Manasypov R; M; , Politova N; V; , Kopysov S; G; , Dara O; M; , Auda Y; , Shirokova L; S; , Kolesnichenko L; G; , Zemtsov V; A; , Kirpotin S; N
刊名: Hydrology and Earth System Sciences
ISSN: 10275606
出版年: 2017
卷: 21, 期:11
起始页码: 5725
结束页码: 5746
语种: 英语
Scopus关键词: Atmospheric aerosols ; Atmospheric chemistry ; Cadmium ; Calcium ; Cesium ; Cluster analysis ; Copper ; Deposition ; Dissolution ; Heavy metals ; Hierarchical systems ; Landforms ; Lithology ; Minerals ; Nickel ; Permafrost ; Principal component analysis ; Rivers ; Silicate minerals ; Silicates ; Snow ; Surface waters ; Atmospheric heavy metals ; Chemical compositions ; Current estimation ; Hierarchical cluster analysis ; Latitudinal gradients ; Major and trace elements ; Particulate fraction ; Winter precipitation ; Trace elements ; chemical composition ; cluster analysis ; concentration (composition) ; flood ; hydrochemistry ; latitudinal gradient ; permafrost ; principal component analysis ; quantitative analysis ; river water ; snow accumulation ; thermokarst ; trace element ; Asia ; Russian Federation ; Siberian Lowland
英文摘要: In order to better understand the chemical composition of snow and its impact on surface water hydrochemistry in the poorly studied Western Siberia Lowland (WSL), the surface layer of snow was sampled in February 2014 across a 1700'km latitudinal gradient (ca. 56.5 to 68°'N). We aimed at assessing the latitudinal effect on both dissolved and particulate forms of elements in snow and quantifying the impact of atmospheric input to element storage and export fluxes in inland waters of the WSL. The concentration of dissolved+colloidal (<'0.45'μm) Fe, Co, Cu, As and La increased by a factor of 2 to 5 north of 63°'N compared to southern regions. The pH and dissolved Ca, Mg, Sr, Mo and U in snow water increased with the rise in concentrations of particulate fraction (PF). Principal component analyses of major and trace element concentrations in both dissolved and particulate fractions revealed two factors not linked to the latitude. A hierarchical cluster analysis yielded several groups of elements that originated from alumino-silicate mineral matrix, carbonate minerals and marine aerosols or belonging to volatile atmospheric heavy metals, labile elements from weatherable minerals and nutrients. The main sources of mineral components in PF are desert and semi-desert regions of central Asia.

The snow water concentrations of DIC, Cl, SO4, Mg, Ca, Cr, Co, Ni, Cu, Mo, Cd, Sb, Cs, W, Pb and U exceeded or were comparable with springtime concentrations in thermokarst lakes of the permafrost-affected WSL zone. The springtime river fluxes of DIC, Cl, SO4, Na, Mg, Ca, Rb, Cs, metals (Cr, Co, Ni, Cu, Zn, Cd, Pb), metalloids (As, Sb), Mo and U in the discontinuous to continuous permafrost zone (64-68°'N) can be explained solely by melting of accumulated snow. The impact of snow deposition on riverine fluxes of elements strongly increased northward, in discontinuous and continuous permafrost zones of frozen peat bogs. This was consistent with the decrease in the impact of rock lithology on river chemical composition in the permafrost zone of the WSL, relative to the permafrost-free regions. Therefore, the present study demonstrates significant and previously underestimated atmospheric input of many major and trace elements to their riverine fluxes during spring floods. A broader impact of this result is that current estimations of river water fluxes response to climate warming in high latitudes may be unwarranted without detailed analysis of winter precipitation. © Author(s) 2017.
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被引频次[WOS]:38   [查看WOS记录]     [查看WOS中相关记录]
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/78996
Appears in Collections:气候变化事实与影响

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作者单位: Shirshov Institute of Oceanology RAS, 36 Nakhimovsky Pr, Moscow, Russian Federation; Geosciences Environment Toulouse, CNRS, University of Toulouse, 14 Avenue Edouard Belin, Toulouse, France; BIO-GEO-CLIM Laboratory, Tomsk State University, 36 Lenina, Tomsk, Russian Federation; N. Laverov Federal Center for Integrated Arctic Research, IEPS, Russian Academy of Science, Arkhangelsk, Russian Federation

Recommended Citation:
Shevchenko V,P,, Pokrovsky O,et al. Impact of snow deposition on major and trace element concentrations and elementary fluxes in surface waters of the Western Siberian Lowland across a 1700'km latitudinal gradient[J]. Hydrology and Earth System Sciences,2017-01-01,21(11)
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