DOI: 10.1016/j.atmosenv.2014.07.012
Scopus记录号: 2-s2.0-84904251603
论文题名: A highly spatially resolved GIS-based model to assess the isoprenoid emissions from key Italian ecosystems
作者: Pacheco C ; K ; , Fares S ; , Ciccioli P
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2014
卷: 96 起始页码: 50
结束页码: 60
语种: 英语
英文关键词: BVOC inventory
; Isoprene
; Isoprenoids
; Italian forests
; Monoterpenes
Scopus关键词: Air pollution
; Atmospheric composition
; Budget control
; Condensation reactions
; Geographic information systems
; Isoprene
; Monoterpenes
; Vegetation
; Biogenic volatile organic compounds
; BVOC inventory
; Isoprenoids
; Italian forests
; Laboratory experiments
; Photochemical pollution
; Spatial and temporal resolutions
; Terrestrial vegetation
; Lipids
; alpha phellandrene
; alpha thujene
; beta farnesene
; beta phellandrene
; beta pinene
; camphene
; caryophyllene
; cineole
; germacrene
; isoprene
; isoprenoid
; limonene
; linalool
; myrcene
; ozone
; para cymene
; pinene
; sabinene
; terpene
; terpinene
; terpineol
; terpinolene
; tricyclene
; unclassified drug
; volatile organic compound
; biogenic emission
; GIS
; isoprenoid
; mapping
; vegetation cover
; volatile organic compound
; article
; circadian rhythm
; ecosystem
; Fagus sylvatica
; geographic information system
; Italy
; land use
; oak
; pine
; Pinus halepensis
; pinus nigra
; Pinus pinea
; Populus nigra
; priority journal
; Quercus ilex
; Quercus petrea
; quercus pubescens
; quercus robur
; Quercus suber
; scots pine
; temperature
; Italy
Scopus学科分类: Environmental Science: Water Science and Technology
; Earth and Planetary Sciences: Earth-Surface Processes
; Environmental Science: Environmental Chemistry
英文摘要: The amount of Biogenic Volatile Organic Compounds (BVOC) emitted from terrestrial vegetation is of great importance in atmospheric reactivity, particularly for ozone-forming reactions and as condensation nuclei in aerosol formation and growth. This work presents a detailed inventory of isoprenoid emissions from vegetation in Italy using an original approach which combines state of the art models to estimate the species-specific isoprenoid emissions and a Geographic Information System (GIS) where emissions are spatially represented. Isoprenoid species and basal emission factors were obtained by combining results from laboratory experiments with those published in literature. For the first time, our investigation was not only restricted to isoprene and total monoterpenes, but our goal was to provide maps of isoprene and individual monoterpenes at a high-spatial (~1km2) and temporal resolution (daily runs, monthly trends in emissions are discussed in the text). Another novelty in our research was the inclusion of the effects of phenology on plant emissions. Our results show that: a) isoprene, a-pinene, sabinene and b-pinene are the most important compounds emitted from vegetation in Italy; b) annual biogenic isoprene and monoterpene fluxes for the year 2006 were ~31.30Gg and ~37.70Gg, respectively; and c) Quercus pubescens+Quercus petrea+Quercus robur, Quercus ilex, Quercus suber and Fagus sylvatica are the principal isoprenoid emitting species in the country. The high spatial and temporal resolution, combined with the species-specific emission output, makes the model particularly suitable for assessing local budgets, and for modeling photochemical pollution in Italy. © 2014 Elsevier Ltd.
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/81216
Appears in Collections: 气候变化事实与影响
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作者单位: Department for Innovation in Biological, Agro-Food and Forest Systems (DIBAF), University of Tuscia, Viterbo, Italy; Institute of Agro-Environmental and Forest Biology, Area della Ricerca del C.N.R., Roma, Italy; Consiglio per la Ricerca e la Sperimentazione in Agricoltura (CRA), Research Center for the Soil-Plant System, 00184 Rome, Italy; Istituto di Metodologie Chimiche (IMC), Area della Ricerca del C.N.R., Roma, Italy
Recommended Citation:
Pacheco C,K,, Fares S,et al. A highly spatially resolved GIS-based model to assess the isoprenoid emissions from key Italian ecosystems[J]. Atmospheric Environment,2014-01-01,96