DOI: 10.1016/j.atmosenv.2014.08.067
Scopus记录号: 2-s2.0-84906771901
论文题名: Inter-comparison between HERMESv2.0 and TNO-MACC-II emission data using the CALIOPE air quality system (Spain)
作者: Guevara M ; , Pay M ; T ; , Martínez F ; , Soret A ; , Denier van der Gon H ; , Baldasano J ; M
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2014
卷: 98 起始页码: 134
结束页码: 145
语种: 英语
英文关键词: Air quality
; Bottom-up emission model
; Downscaled methodology
; Emissions
; Urban scale
Scopus关键词: Air quality
; Dust
; Nitrogen oxides
; Ozone
; Particulate emissions
; Sulfur dioxide
; Particulate emissions
; Agricultural operations
; Air quality systems
; Downscaled methodology
; Emission inventories
; Emission model
; International shippings
; Residential emissions
; Urban scale
; Emission data
; Intercomparisons
; Industrial emissions
; Air quality
; nitrogen dioxide
; ozone
; sulfur dioxide
; air quality
; comparative study
; concentration (composition)
; estimation method
; industrial emission
; urban pollution
; coast
; data set
; dust
; emission inventory
; nitrogen dioxide
; ozone
; resuspension
; road
; sulfur dioxide
; air analysis
; air pollutant
; air quality
; air quality control
; article
; comparative study
; concentration (parameters)
; industrial area
; intermethod comparison
; methodology
; observational study
; particulate matter
; priority journal
; rural area
; simulation
; Spain
; summer
; time series analysis
; urban area
; winter
; air monitoring
; air quality
; Article
; controlled study
; dust
; environmental impact
; exhaust gas
; high elective resolution modelling emission system
; information processing
; intermethod comparison
; noise measurement
; residential area
; shipping
; tno macc ii emission inventory
; traffic noise
; Spain
Scopus学科分类: Environmental Science: Water Science and Technology
; Earth and Planetary Sciences: Earth-Surface Processes
; Environmental Science: Environmental Chemistry
英文摘要: This work examines and compares the performance of two emission datasets on modelling air quality concentrations for Spain: (i) the High-Elective Resolution Modelling Emissions System (HERMESv2.0) and (ii) the TNO-MACC-II emission inventory. For this purpose, the air quality system CALIOPE-AQFS (WRF-ARW/CMAQ/BSC-DREAM8b) was run over Spain for February and June 2009 using the two emission datasets (4km×4km and 1h). Nitrogen dioxide (NO2), sulphur dioxide (SO2), Ozone (O3) and particular matter (PM10) modelled concentrations were compared with measurements at different type of air quality stations (i.e. rural background, urban, suburban industrial). A preliminary emission comparison showed significant discrepancies between the two datasets, highlighting an overestimation of industrial emissions in urban areas when using TNO-MACC-II. However, simulations showed similar performances of both emission datasets in terms of air quality. Modelled NO2 concentrations were similar between both datasets at the background stations, although TNO-MACC-II presented lower underestimations due to differences in industrial, other mobile sources and residential emissions. At Madrid urban stations NO2 was significantly underestimated in both cases despite the fact that HERMESv2.0 estimates traffic emissions using a more local information and detailed methodology. This NO2 underestimation problem was not found in Barcelona due to the influence of international shipping emissions located in the coastline. An inadequate characterization of some TNO-MACC-II's point sources led to high SO2 biases at industrial stations, especially in northwest Spain where large facilities are grouped. In general, surface O3 was overestimated regardless of the emission dataset used, depicting the problematic of CMAQ on overestimating low ozone at night. On the other hand, modelled PM10 concentrations were less underestimated in urban areas when applying HERMESv2.0 due to the inclusion of road dust resuspension, whereas the underestimation at suburban industrial stations indicated deficiencies in fugitive emission sources characterization (agricultural operations, windblown dust emissions). © 2014 Elsevier Ltd. Citation statistics:
资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/81238
Appears in Collections: 气候变化事实与影响
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作者单位: Barcelona Supercomputing Center - Centro Nacional de Supercomputación (BSC-CNS), Earth Sciences Department, Jordi Girona 29, Edificio Nexus II, 08034 Barcelona, Spain; TNO Department Climate Air, and Sustainability, Utrecht, Netherlands; Environmental Modelling Laboratory, Technical University of Catalonia, Avda. Diagonal 647, Edificio H, Oficina 10.23, 08028 Barcelona, Spain
Recommended Citation:
Guevara M,, Pay M,T,et al. Inter-comparison between HERMESv2.0 and TNO-MACC-II emission data using the CALIOPE air quality system (Spain)[J]. Atmospheric Environment,2014-01-01,98