Air pollution
; Air quality
; Boundary layers
; Carbon
; Carbon dioxide
; Mixing
; Nitrates
; Aerosol nitrates
; Air quality impacts
; Chemical production
; Cloud-topped boundary layer
; Fine particulate matter
; Nighttime temperatures
; Particle number concentration
; Stagnation
; Pollution
; ammonium nitrate
; black carbon
; carbon dioxide
; aerosol
; air quality
; atmospheric pollution
; boundary layer
; chemical pollutant
; cloud
; cold pool
; mixing
; nitrate
; stagnation flow
; winter
; aerosol
; air pollutant
; air pollution
; air quality
; Article
; cloud
; cold climate
; low level cloud
; meteorology
; particulate matter
; priority journal
; surface property
; swimming pool
; winter
; United States
; Washington [United States]
; Yakima County
Scopus学科分类:
Environmental Science: Water Science and Technology
; Earth and Planetary Sciences: Earth-Surface Processes
; Environmental Science: Environmental Chemistry
英文摘要:
The Yakima Air Wintertime Nitrate Study (YAWNS) was conducted in January 2013 to investigate the drivers of elevated levels of fine particulate matter (PM2.5) frequently present in the region during winter stagnation periods. An extended stagnation period occurred during the study. For the first four days of the event, skies were clear and the strong diel variation in air pollution patterns were consistent with the expected effects of strong low-level nighttime temperature inversions with moderate mixing during daylight hours. Later in the event a low-level cloud layer formed that persisted over the Yakima Valley for the next seven days while regional conditions remained stagnant. Coincident with the onset of cloud, the levels of all measured primary pollutants, including CO2, CO, NOx, particle number concentration, and black carbon, dropped dramatically and remained low with negligible diel variation for as long as the cloud layer was present. The observed patterns for these air pollutants are consistent with decreased stability and enhanced mixing associated with the cloud-topped boundary layer. Interestingly, levels of secondary pollutants, most notably particulate ammonium nitrate, did not exhibit the same decline. This difference may be due to shifts in the chemical production of secondary pollutants during cloudy conditions, or may merely reflect a further influence of mixing. The results imply that the best strategies for managing wintertime air quality during episodes of persistent cloud are likely different from those needed during clear-sky stagnation events. � 2017
Laboratory for Atmospheric Research, Department of Civil & Environmental Engineering, Washington State University, United States; Washington Department of Ecology, United States; Gene and Linda Voiland School of Chemical Engineering and Bioengineering, Washington State University, United States; Department of Geological Sciences, Central Washington University, United States
Recommended Citation:
VanReken T,M,, Dhammapala R,et al. Role of persistent low-level clouds in mitigating air quality impacts of wintertime cold pool conditions[J]. Atmospheric Environment,2017-01-01,154