globalchange  > 气候变化事实与影响
DOI: 10.1016/j.atmosenv.2018.01.018
Scopus记录号: 2-s2.0-85041565156
论文题名:
Optical, microphysical and radiative properties of aerosols over a tropical rural site in Kenya, East Africa: Source identification, modification and aerosol type discrimination
作者: Boiyo R; , Kumar K; R; , Zhao T
刊名: Atmospheric Environment
ISSN: 0168-2563
EISSN: 1573-515X
出版年: 2018
卷: 177
起始页码: 234
结束页码: 252
语种: 英语
英文关键词: AERONET ; Aerosol-type classification ; AOD ; East Africa ; Radiative forcing ; SSA
Scopus关键词: Atmospheric aerosols ; Atmospheric radiation ; Climate change ; Heat radiation ; Optical properties ; Refractive index ; Rural areas ; Sea level ; AERONET ; Aerosol direct radiative forcing ; Aerosol optical property ; Aerosol robotic networks ; Aerosol types ; East Africa ; Radiative forcings ; Single scattering albedo ; Aerosols
Scopus学科分类: Environmental Science: Water Science and Technology ; Earth and Planetary Sciences: Earth-Surface Processes ; Environmental Science: Environmental Chemistry
英文摘要: A better understanding of aerosol optical, microphysical and radiative properties is a crucial challenge for climate change studies. In the present study, column-integrated aerosol optical and radiative properties observed at a rural site, Mbita (0.42°S, 34.20 °E, and 1125 m above sea level) located in Kenya, East Africa (EA) are investigated using ground-based Aerosol Robotic Network (AERONET) data retrieved during January, 2007 to December, 2015. The annual mean aerosol optical depth (AOD500 nm), Ångström exponent (AE440–870 nm), fine mode fraction of AOD500 nm (FMF500 nm), and columnar water vapor (CWV, cm) were found to be 0.23 ± 0.08, 1.01 ± 0.16, 0.60 ± 0.07, and 2.72 ± 0.20, respectively. The aerosol optical properties exhibited a unimodal distribution with substantial seasonal heterogeneity in their peak values being low (high) during the local wet (dry) seasons. The observed data showed that Mbita and its environs are significantly influenced by various types of aerosols, with biomass burning and/or urban-industrial (BUI), mixed (MXD), and desert dust (DDT) aerosol types contributing to 37.72%, 32.81%, and 1.40%, respectively during the local dry season (JJA). The aerosol volume size distribution (VSD) exhibited bimodal lognormal structure with a geometric mean radius of 0.15 μm and 3.86–5.06 μm for fine- and coarse-mode aerosols, respectively. Further, analysis of single scattering albedo (SSA), asymmetry parameter (ASY) and refractive index (RI) revealed dominance of fine-mode absorbing aerosols during JJA. The averaged aerosol direct radiative forcing (ARF) retrieved from the AERONET showed a strong cooling effect at the bottom of the atmosphere (BOA) and significant warming within the atmosphere (ATM), representing the important role of aerosols played in this rural site of Kenya. Finally, the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model revealed that aerosols from distinct sources resulted in enhanced loading during JJA. © 2018 Elsevier Ltd
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资源类型: 期刊论文
标识符: http://119.78.100.158/handle/2HF3EXSE/83018
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作者单位: Collaborative Innovation Centre on Forecast and Evaluation of Meteorological Disasters, Key Laboratory of Meteorological Disaster, Ministry of Education (KLME), International Joint Laboratory on Climate and Environment Change (ILCEC), Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, School of Atmospheric Physics, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China; Department of Physical Sciences, Meru University of Science and Technology, P.O. Box 972-60200, Meru, Kenya

Recommended Citation:
Boiyo R,, Kumar K,R,et al. Optical, microphysical and radiative properties of aerosols over a tropical rural site in Kenya, East Africa: Source identification, modification and aerosol type discrimination[J]. Atmospheric Environment,2018-01-01,177
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