项目编号: | 1705864
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项目名称: | SusChEM: Ultrafine Particle Formation in Advanced Low Carbon Combustion Processes |
作者: | Pratim Biswas
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承担单位: | Washington University
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批准年: | 2017
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开始日期: | 2017-06-01
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结束日期: | 2021-05-31
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资助金额: | 499841
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资助来源: | US-NSF
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项目类别: | Standard Grant
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国家: | US
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语种: | 英语
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特色学科分类: | Engineering - Chemical, Bioengineering, Environmental, and Transport Systems
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英文关键词: | ultrafine particle formation
; low-carbon
; resultant formation
; conventional combustion
; pressurized oxycombustion system
; pressurized oxy-combustion
; next-generation low-carbon combustion technology
; advanced low-carbon combustion process
; char combustion
; fuel particle
; carbon intensity
; fine particle
; combustion condition
; combustion science
; carbon capture technology
; advanced combustion process
; particle formation
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英文摘要: | 1705864 Biswas, Pratim
One area that is critical to advancement of carbon capture technologies is understanding ultrafine particle formation under combustion conditions associated with next-generation low-carbon combustion technologies, such as pressurized oxy-combustion. Another area where ultrafine particle formation is of interest is that of co-firing coal with natural gas (NG), as this can reduce the carbon intensity of existing coal-fired power plants. A thorough understanding of ultrafine particle formation is essential to both predict and control radiation in boilers and to avoid the deleterious effects of fine particles on fouling in the boilers and emissions in the atmosphere. To this end, three universities have joined forces to utilize their unique capabilities in the fields of aerosol and combustion science to address this topic.
The research will address the following hypotheses, which are focused on particle formation, evolution, and measurement in environments conducive to advanced low-carbon combustion processes: (1)The high CO2 concentrations, elevated pressures and high oxygen concentrations of these processes, relative to conventional combustion, will affect the heating rate, temperature and environment of the fuel during pyrolysis and char combustion, thus affecting the volatilization of inorganic mineral species and the subsequent ultrafine particle formation and growth; (2) The interaction of organic constituents with the inorganic mineral matter in pressurized oxycombustion systems will affect the chemical reaction pathways and resultant formation, growth and transformation of soot and organic aerosols; (3) During NG co-firing with coal, the change in the local chemical environment of the fuel particle will affect ultrafine particle formation; (4) Multiscale models ranging from ab-initio to meso- to full-scale can be validated with a range of instrumentation used in controlled experiments, and will aid in the overall understanding of ultrafine particle formation in advanced combustion processes. This award is co-funded by the CBET Environmental Sustainability program and the Office of International Science and Engineering. |
资源类型: | 项目
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标识符: | http://119.78.100.158/handle/2HF3EXSE/90171
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Appears in Collections: | 全球变化的国际研究计划 科学计划与规划
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Recommended Citation: |
Pratim Biswas. SusChEM: Ultrafine Particle Formation in Advanced Low Carbon Combustion Processes. 2017-01-01.
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