globalchange  > 全球变化的国际研究计划
项目编号: 1552086
项目名称:
Collaborative Research: Formation of Organic Nitrogen and Secondary Organic Aerosol Related to Nitrate Radical Oxidation of Volatile Organic Compounds
作者: Robert Griffin
承担单位: William Marsh Rice University
批准年: 2016
开始日期: 2016-02-15
结束日期: 2019-01-31
资助金额: 238544
资助来源: US-NSF
项目类别: Standard Grant
国家: US
语种: 英语
特色学科分类: Geosciences - Atmospheric and Geospace Sciences
英文关键词: volatile organic carbon ; particulate organic nitrate ; oxidation ; oxidation state ; forest ; soa ; soa formation ; impact nitrogen oxide ; nitrogen species ; ambient aerosol
英文摘要: This project focuses on increasing the understanding of how human-produced emissions combine with biogenic emissions from forests to influence the formation of small particles in the atmosphere. A mobile laboratory will be deployed to two different types of forests (urban and remote) in order to compare and contrast the impact of long-range and short-range transport of nitrogen species to forests. The results will lead to improved control strategies that minimize the health, visibility and climate effects of anthropogenic emissions.

The primary objectives of the science campaign are to: (1) Characterize the ambient aerosol, radiation, and trace gases at two forest sites, both above and below the canopy, and along a north-south transect in the central United States; (2) Quantify the level of oxidation found in SOA using atomic ratios (such as the oxygen to carbon ratio, O:C) and determine the impact the presence of particulate organic nitrate (PON) has on the observed oxidation state of the submicron particulate matter (PM); (3) Investigate how in-canopy gradients and through-canopy transport impact submicron PM, PON, and oxidants; (4) Determine the impact nitrogen oxides (NOx) have on volatile organic carbon (VOC) oxidation and SOA formation in all locations; (5) Compare and contrast the chemistry of remote, on-road, and urban forested areas; (6) Identify the factors contributing to SOA using positive matrix factorization (PMF) to identify important components of SOA under different levels of anthropogenic influence both above and below canopy; and (7) Investigate the fate of NOx in all locations.
资源类型: 项目
标识符: http://119.78.100.158/handle/2HF3EXSE/92857
Appears in Collections:全球变化的国际研究计划
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Robert Griffin. Collaborative Research: Formation of Organic Nitrogen and Secondary Organic Aerosol Related to Nitrate Radical Oxidation of Volatile Organic Compounds. 2016-01-01.
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